The original idea was to harvest the carbon for the sake of simultaneously terraforming a CO2 rich atmosphere and gaining industrial benefit from doing so in the form of carbon based materials. My initial thoughts included nanotube based armors and building materials, but plastics, synthetic fossil fuels... just about anything could be a final outcome.
The advantage of a mechanical means rather than a biological means is that it could more easily be adapted to other elements/molecules for different atmospheres, then a different "production module" attached to make whatever is intended.
I *LIKE* this idea. The problem with using Earth plants is they need water and only operate well in a narrow range of temperatures. (One reasohy greening the Sahara in a Global Warming world is dubious.) However, algae are self replicating and VERY efficient.
I've always liked the idea of cyborg lichen. Build nanotube and silicate "body armor" for algae. Combine nanomachines and lichen.
There are lighter then air aerogels...embed algae and solar powered nanomachines in a lighter then air aerogel and let it float high in the atmosphere above the clouds. On venus it could reflect away excess sunlight, to